環(huán)境催化與污染控制化學團隊
學術帶頭人：唐和清
團隊成員：
唐和清,、呂康樂、王成俊,、李立忠,、張勝花,、丁耀彬,、雷鳴、萬震
團隊簡介：
本團隊一直致力于研究環(huán)境中典型污染物的賦存形態(tài),、分布規(guī)律,、光化學轉化行為歸趨以及環(huán)境催化新材料及其在污染控制中的應用，尤其在高性能環(huán)境催化材料的設計,、可控制備,、性能研究以及應用等方面取得了創(chuàng)新性的研究成果。
主要研究方向：
●污染控制化學：主要包括類Fenton體系的擴展與強化,、微污染水體系的深度凈化,、工業(yè)污染水與固廢的處置；
●多功能催化劑：重點研究具有強吸附能力的催化性雙功能材料,，包括以粘土礦物,、多形態(tài)碳等基質的多功能材料；
●光催化：重點研究二氧化鈦及新型光催化材料的可控制備,，及其降解污染物的反應歷程和催化機理,；
●分子印跡：重點研究分子印跡型吸附材料及其與二氧化鈦復合而成的選擇性光催化材料，開發(fā)其在環(huán)境污染控制應用,；
●環(huán)境光化學：重點研究地表水及大氣中持久性有機污染物的賦存形態(tài),、分布規(guī)律、光化學轉化及行為歸趨
●湖泊生態(tài)修復：重點研究富營養(yǎng)化湖泊的生態(tài)響應過程,、進程,、機理以及防控措施。
近期完成或正在進行的主要研究項目：
1.國家自然科學基金面上項目,，載流子自分離型光催化微界面的構筑及其高效降解溴酚類污染物（21876209）.
2.國家自然科學基金面上項目,，“C8”類全氟化合物固廢的機械化學無害化處置及資源化方法研究（21777194）.
3.國家自然科學基金面上項目,，基于晶面接觸效應構建高效半導體復合光催化材料（51672312）.
4.國家自然科學基金面上項目，天然水中鄰苯二甲酸酯類塑化劑的富存與光降解機理研究(21477088).
5.國家自然科學基金面上項目,，催化反應性超級吸附體系的構筑及其去除低暴露水平環(huán)境激素污染物的研究（21377169）.
6.國家自然科學基金面上項目,，基于生物原細胞模型的凝聚層半導體光催化體系研究（21373275）.
7.國家自然科學基金面上項目，微界面調(diào)控增強全氟羧酸化學催化氧化降解的方法研究（21077037）.
8.國家自然科學基金面上項目,，高能面二氧化鈦的超強氟效應光催化降解惡臭有毒氣體（20977114）.
9.國家自然科學基金面上項目,，人工抗體型光催化劑的合成及選擇性降解有毒污染物研究（20677019）.
10.國家自然科學基金地區(qū)項目：滇池水華優(yōu)勢藍藻的磷吸收存儲及水華消亡時殘體的磷礦化機制（51468066）.
11.國家自然科學基金青年項目，In2O3表面活性氫物種調(diào)控及其實現(xiàn)PBDEs光催化深度脫溴的反應機制研究（21906184）
11.國家自然科學基金青年項目,，g-C3N4固載的單原子分散Pd催化劑及其催化PBDEs深度還原脫溴（21707170）.
11.國家自然科學基金青年項目,，自摻雜鉍基光催化劑光催化氧化及其單線態(tài)氧直接氧化協(xié)同降解PPCPs（21507168）.
12.國家自然科學基金青年項目，天然酚類抗氧化劑對果蔬表面二噻農(nóng)殺菌劑光化學轉化的影響及其機理研究(21207102).
13.國家自然科學基金青年項目,，滇池水華優(yōu)勢藍藻的磷吸收存儲及水華消亡時殘體的磷礦化機制（51468066）.
13.國家863計劃項目子課題,，集約養(yǎng)殖外源化學品污染控制技術（2012AA06A304）.
14.教育部“新世紀優(yōu)秀人才支持計劃”，空心納米顆粒自組裝二氧化鈦空心微球光催化空氣凈化（NCET-12-0668）,，2013-2015.
15.湖北省杰出青年基金,，橄欖球形單晶二氧化鈦空心球的制備與光催化性能研究（2011CDA107）.
近期代表性研究論文：
1. Chao Yang, Qiuyan Tan, Qin Li, Jie Zhou*, Jiajie Fan, Bing Li, Jie Sun, Kangle Lv*, 2D/2D Ti3C2 MXene/g-C3N4 nanosheets heterojunction for high efficient CO2 reduction photocatalyst: Dual effects of urea, Appl. Catal. B: Environ. 2020, 268, 118738. （ESI高被引）
2. Xiaofang Li, Zhao Hu, Qin Li, Ming Lei, Jiajie Fan, Sónia A.C. Carabineiro, Yi Liu*, Kangle Lv*, Three in one: atomically dispersed Na boosting the photoreactivity of carbon nitride towards NO oxidation, Chem. Commun. 2020, DOI: 10.1039/d0cc05948j.
3. Zhao Hu, Xiaofang Li*, Sushu Zhang, Qin Li, Jiajie Fan, Xianlin Qu, Kangle Lv*, Fe1/TiO2 hollow microspheres: Fe and Ti dual active sites boosting the photocatalytic oxidation of NO, Small 2020, 2004583.
4. Zhao Hu, Chao Yang, Kangle Lv*, Qin Li, Xiaofang Li, Jiajie Fan, Single atomic Au induced dramatic promotion of the photocatalytic activity of TiO2 hollow microspheres, Chem. Commun.2020, 56, 1745-1748.
5. Ming Lei, Zhiying Wang, Yao Tang, Huimin Wang, Lihua Zhu*, Heqing Tang*, Peculiar and full debromination of tetrabromodiphenyl ether on Pd/TiO2: a competing route through hydro-debromination and coupling-debromination, Appl. Catal. B: Environ., 2020, 275, 119093.
6. Ming Lei, Zhiying Wang, Lihua Zhu*, Wenshan Nie, Heqing Tang*, Complete debromination of 2,2’,4,4’-tetrabromodiphenyl ether by visible-light photocatalysis on g-C3N4 supported Pd, Appl. Catal. B: Environ., 2020, 261, 118236.
7. Shun Guo, Lihua Zhu*, Tetsuro Majima, Ming Lei, Heqing Tang*, Reductive debromination of polybrominated diphenyl ethers: dependence on Br number of the Br-rich phenyl ring. Environ. Sci. Technol., 2019, 53, 8, 4433-4439.
8. Nan Wang, Hanqing Lv, Yuqi Zhou, Lihua Zhu*, Yue Hu, Tetsuro Majima, Heqing Tang*, Complete defluorination and mineralization of perfluorooctanoic acid by a mechanochemical method using alumina and persulfate. Environ. Sci. Technol., 2019, 53, 14, 8302-8313.
9. Jin Cao, Wenshan Nie, Long Huang, Yaobin Ding*, Kangle Lv, Heqing Tang*, Photocatalytic activation of sulfite by nitrogen vacancy modified graphitic carbon nitride for efficient degradation of carbamazepine, Appl. Catal. B: Environ., 2019, 241, 18-27. （ESI高被引）
10. Jinshui Cheng, Zhao Hu, Qin Li, Xiaofang Li*, Shun Fang, Xiaofeng Wu, Mei Li, Yaobin Ding, Bing Liu, Changjun Yang, Lili Wen, Yi Liu, Kangle Lv*, Fabrication of high photoreactive carbon nitride nanosheets by polymerization of amidinourea for hydrogen production, Appl. Catal. B: Environ.2019, 245, 197-206.
11. Chao Yang, Qin Li*, Yang Xia, Kangle Lv*, Mei Li, Enhanced visible-light photocatalytic CO2 reduction performance of Znln2S4 microspheres by using CeO2 as cocatalyst, Appl. Surf. Sci.2019, 464, 388-395. （ESI高被引）
12. Wenshan Nie, Qihang Mao, Yaobin Ding*, Yue Hu, Heqing Tang*, Highly efficient catalysis of chalcopyrite with surface bonded ferrous species for activation of peroxymonosulfate toward degradation of bisphenol A: A mechanism study. J. Hazard. Mater., 2019, 364, 59-68. （ESI高被引）
13. Jingsha. Xu, Chunrong. Jia, Jun. He*, Honghui. Xu, Yuting. Tang, Ddongsheng. Ji, Huan. Yu, Hang. Xiao, Chengjun Wang*, Biomass burning and fungal spores as sources of fine aerosols in Yangtze River Delta, China-using multiple organic tracers to understand variability, correlations and origins. Environmental Pollution, 2019, 251, 155-165.
14. Yuhan Li, Xiaofeng Wu, Wingkei Ho*, Kangle Lv*, Qin Li, Mei Li, Shuncheng Lee, Graphene-induced formation of visible-light-responsive SnO2-Zn2SnO4 Z-scheme photocatalyst with surface vacancy for the enhanced photoreactivity towards NO and acetone oxidation, Chem. Eng. J.2018, 336, 200-210. （ESI高被引）
15. Ming Lei, Shun Guo, Zhiying Wang, Lihua Zhu*,Heqing Tang*, Ultrarapid and deep debromination of tetrabromodiphenyl ether over noble-metal-free Cu/TiO2 nanocomposites under mild conditions. Environ. Sci. Technol., 2018, 52, 20, 11743-11751.
16. Yuhan Li, Kangle Lv*, Wingkei Ho*, Fan Dong, Xiaofeng Wu, Yang Xia, Hybridization of rutile TiO2 (rTiO2) with g-C3N4 quantum dots (CN QDs): An efficient visible-light-driven Z-scheme hybridized photocatalyst. Appl. Catal. B: Environ.2017, 202, 611-619. （ESI高被引）
17.Yaobin Ding, Guangli Zhang, Xueru Wang, Lihua Zhu*, Heqing Tang*, Chemical and photocatalytic oxidative degradation of carbamazepine by using metastable Bi3+ self-doped NaBiO3 nanosheets as a bifunctional material, Appl. Catal. B: Environ. 2017, 202, 528-838.
18. Ruiwen Yang, Jinghua Cai, Kangle Lv*, Xiaofeng Wu, Wenguang Wang, Zhihua Xu, Mei Li*, Qin Li, Weiqing Xu, Fabrication of TiO2 Hollow Microspheres Assembly from Nanosheets (TiO2-HMSs-NSs) with Enhanced Photoelectric Conversion Efficiency in DSSCs and Photocatalytic Activity. Appl. Catal. B: Environ. 2017,210, 184-193.
19. Kangle Lv*, Xiaojia Guo, Xiaofeng Wu, Qin Li, Wingkei Ho*, Mei Li, Hengpeng Ye, Dongyun Du, Photocatalytic selective oxidation of phenol to produce dihydroxybenzenes in a TiO2/UV system: Hydroxyl radical versus hole. Appl. Catal. B: Environ. 2016, 199, 405-411.
20. Shun Fang, Yang Xia, Kangle Lv*, Qin Li, Jie Sun, Mei Li*, Effect of carbon-dots modification on the structure and photocatalytic activity of g-C3N4. Appl. Catal. B: Environ. 2016, 185, 225-232.
21. Shun Fang, Yang Xia, Kangle Lv*, Qin Li, Jie Sun, Mei Li*, Effect of carbon-dots modification on the structure and photocatalytic activity of g-C3N4. Appl. Catal. B: Environ. 2016, 185, 225-232. （ESI高被引）
22. Ze’ai Huang, Qiong Sun, Kangle Lv*, Zehui Zhang, Mei Li, Bing Li, Effect of contact interface between TiO2 and g-C3N4 on the photoreactivity of g-C3N4/TiO2 photocatalyst: (001) vs (101) facets of TiO2. Appl. Catal. B: Environ.2015, 164, 420-427. （ESI高被引）
23. Xiaobo Wang, Yanlei Qin, Lihua Zhu, and Heqing Tang*, Nitrogen-Doped Reduced Graphene Oxide as a Bifunctional Material for Removing Bisphenols: Synergistic Effect between Adsorption and Catalysis, Environ. Sci. Technol.2015, 49, 11, 6855–6864. （ESI高被引）
24. Yaobin Ding, Fan Yang, Lihua Zhu*, Nan Wang, Heqing Tang*, Bi3+ self doped NaBiO3 nanosheets: Facile controlled synthesis and enhanced visible light photocatalytic activity, Appl. Catal. B: Environ. 2015, 164, 151-158.
